Effective triclosan removal by using porous aromatic frameworks in continuous fixed-bed column studies.

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  • Author(s): Li Y;Li Y;Li Y; Gong F; Gong F; Yang W; Yang W; Liu B; Liu B
  • Source:
    Environmental science and pollution research international [Environ Sci Pollut Res Int] 2023 Dec; Vol. 30 (57), pp. 121007-121013. Date of Electronic Publication: 2023 Nov 10.
  • Publication Type:
    Journal Article
  • Language:
    English
  • Additional Information
    • Source:
      Publisher: Springer Country of Publication: Germany NLM ID: 9441769 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1614-7499 (Electronic) Linking ISSN: 09441344 NLM ISO Abbreviation: Environ Sci Pollut Res Int Subsets: MEDLINE
    • Publication Information:
      Publication: <2013->: Berlin : Springer
      Original Publication: Landsberg, Germany : Ecomed
    • Subject Terms:
      Triclosan* ; Water Pollutants, Chemical* ; Water Purification*; Porosity ; Adsorption ; Water
    • Abstract:
      Triclosan (TCS) has been regarded as an emerging contaminant in aquatic systems, making its efficient removal of great significance. In this study, NPVMo@iPAF-1, with a specific surface area of 665 m 2 /g, was prepared by incorporating (NH 4 ) 5 H 6 PV 8 Mo 4 O 40 into porous aromatic frameworks (PAF). The maximum adsorption capacity of TCS on NPVMo@iPAF-1 reached 917.1 mg/g, as calculated from the Langmuir model. Fixed-bed columns packed with NPVMo@iPAF-1 were employed for TCS removal; the experiment data strongly correlated with the Thomas and Yoon-Nelson models under different operational conditions. Pore preservation, electrostatic effects, and the synergistic effect of π-π interactions contributed to the effective adsorption of TCS onto NPVMo@iPAF-1. The NPVMo@iPAF-1 fixed-bed column could be effectively regenerated through in-situ ozonation for more than 10 regeneration cycles. NPVMo@iPAF-1 turned out to be a promising adsorbent for removing TCS not only from pure water but also from reclaimed water and surface water samples.
      (© 2023. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.)
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    • Grant Information:
      2412019FZ020 Fundamental Research Funds for the Central Universities; 2021YJSB042 Tianjin Research Innovation Project for Postgraduate Students
    • Contributed Indexing:
      Keywords: Adsorption; Fixed-bed column; In situ regeneration; Porous aromatic frameworks; Reclaimed water; Triclosan
    • Accession Number:
      4NM5039Y5X (Triclosan)
      0 (Water Pollutants, Chemical)
      059QF0KO0R (Water)
    • Publication Date:
      Date Created: 20231110 Date Completed: 20231207 Latest Revision: 20231215
    • Publication Date:
      20231215
    • Accession Number:
      10.1007/s11356-023-30714-2
    • Accession Number:
      37947929