Delocalized, asynchronous, closed-loop discovery of organic laser emitters.

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    • Subject Terms:
      LASERS; SOLID-state lasers; TIME-resolved spectroscopy; ARTIFICIAL intelligence; DELAYED fluorescence
    • Abstract:
      The article focuses on revolutionizing materials discovery through a distributed, AI-guided approach, integrating synthesis, characterization, and testing across multiple geographical sites via a central cloud hub, facilitating global design-make-test-analyze loops for organic solid-state lasers (OSLs). Leveraging iterative Suzuki–Miyaura couplings and a building block–based strategy, the study demonstrates the asynchronous, closed-loop discovery of small-molecule gain materials for OSLs.